I just read Ari Meisel's Less Doing, More Living: Make Everything in Life Easier in one day. Even though I read a lot about productivity and am pretty organized, it still gave me food for thought...and apps to try.
The premise of the book is that 20% of effort begets 80% of the results, so you should only be spending your time on the effective 20%. You do this first by optimizing all your tasks, then automating or outsourcing most of what's left and only doing what no one else can do for you. This is similar to what's been discussed in other books I've read and written about, but he adds a twist.
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